It would seem likely that, the balance being old is Imperial, so the weights would increment a a geometric progression with a factor of 2.
So one of each of: 1/2 oz, 1, 2, 4, 8, 16 would allow items weighing up to 31 1/2 ounces to be measured in 1/2 oz increments. . Duplicating some or all of the weights would extend the range.
Methods of determining the missing weights have already been described, so as long as one weight is available, the others ought to be to be derived by using temporary ones to halve or double them datum weight.
For greater precision the way is to drill and tap a hole and fit a grubscrew. The weight can then be adjusted to the desired level more accurately by adding lead shot under the grubscrew.
This was the method advocated by the local Weights and Measures Inspector when we needed a set of standard weights for calibrating dynamometers. He was apologetic that the 25 and 50 lb weights would not be closer than a few grains!
Howard.