Interesting history. Thanks.
If the engine is one of the inlet-over-exhaust models, the equivalent Harley would be the J Model. If you Google Harley J Model you will find there are numerous forums and a few companies making aftermarket parts, including cams, who may be able to provide cam specs that you could copy. The IOE is pretty specialised as OHV and SV cams usually have different characteristics and this has one of each!
The more you look at it, the less important Lobe Separation Angle would seem to be. All that really matters is valve events: valve opening, valve closing and lift. All the rest is secondary. The LSA will fall wherever it ends up depending on valve opening and closing specs. Keep the valves open longer, the LSA widens. And so on.
Of the secondary considerations, probably the most important would be the flank angles. Steep angles open/close the valves very quickly, holding the valve fully open for as long as possible. This puts great strain on pushrods and rocker arms etc. Gentler flank angles open and close valves gently, running quieter, with less stress, but giving less performance due to valve being not fully open for most of the duration. Looking at J Model cams here https://www.competitiondist.com/products/cam-001-harley-j-jd-cam-gear-1917-1929-61-74-inch it looks like they open fast and close slow, probably to save the soft valve seats of the day before lleaded petrol?
This page here http://www.geocities.ws/pravgeusau/engine.htm gives some cam timing specs for the J Model IOE engine, unfortunately in inches before and after TDC etc. But it is a 3-1/2 inch stroke and there are online calculators that let you convert that into degrees.
“The exhaust valve should start to open about 9/16″ before bottom centre (BBDC) and close 1/32″ after top (ATDC), after 1917, 3/32″ (ATDC). The inlet valves start to open 1/32″ before top (BTDC) and close 1/8″ past bottom (ABDC), after 1917 5/32″ (BTDC) and 3/8” (ABDC).
It was found that although the 1917 and later models have different cams shapes for the front and rear cylinders, the timing is the same for both cylinders. Actually measured values are; exhaust opens 14 mm BBDC and closes 1 mm ATDC. The inlet valve opens 5 mm BTDC and closes 22mm ABDC.”
It looks like there is not much overlap at TDC, indicative of a wide LSA. But a lot of degrees translate to not much linear movement close to TDC so would need to be calculated out to be sure.
Have fun!